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The entire Suikoden series
More JRPG ports especially Tales of Xillia.

Legacy of Kain. Blood Omen

The last of us. I know it's a console exclusive, but so was "I am alive" and it still made it to the pc.
So maybe... it's more than wishful thinking?

Forza Horizon 2.

Mass Effect 3
Uncharted

Freelancer, hands down.

Bloodborne

Radiant Silvergun

HORIZON ZERO DAWN
Dragon Age 2 & Inquisition
Red Dead Redemption 1 & 2
Combat Flight Simulator 1 & 2

A 32-bit, Windows version of Carmen Sandiego games
Probably some others as well

Red Dead Redemption 1 and 2 - but I think it will be released on steam soon. And RDR1 pack will be the biggest feature on PC like FPP mode in GTA V.

To people who wants Playstation exclusives - It's not gonna happen! Sony is not Microsoft so their exclusives will be Playstation exclusives for life.

All Origin exclusives and an old one: Oni.

Megaman Zero
Megaman Zx
Megaman Zxa

Journey. Always wanted to play it.

The Sims 4

Good old Black & White 1 and 2 <3
Loved those games

Multiplayer Games Only ! Any kind !

KH 1/2 as well, more like Birth By Sleep :D

Parasite Eve and Dino Crisis
(I probably already said Xenogears earlier in this thread).

Star Trek Armada 2, with full multiplayer support

Final Fantasy I
Final Fantasy II
Final Fantasy Tactics War of the Lions

Warhammer - Mark of Chaos
as Gold Edition, with Battle March Expansion

https://www.youtube.com/watch?v=AxcQer2jFL8