I would say a lot of it depends on the types of games you like. Mafia 2, Spec Ops: The Line are both solid titles. The Darkness 2 is a fun playthrough as well, IMO. Not been sucked into the Civ world yet, so no opinion there.
Edit
I just glimpsed at your library, looks like the recommendations I made would be your best bet. Mafia 2 is similar to GTA, Spec Ops and Darkness are both decent shooters.
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Civ5 but only if you get it GOTY and with the Gods and Kings expansion, as it changes the whole gameplay for the better, better AI/Combat/Mechanics. Mafia 2 only if you're a fan of the first game, it's a great story-telling game. Spec Ops: The Line seems to have a great story, I heard many great things about it, but average gameplay. Darkness 2 seems to be very fun in all aspects.
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Civ 5 is the best game on the list that offers the most hours of gameplay, but it really depends what you're looking for. If you enjoy GTA-style games the most, go for Mafia 2. If you like shooters, then Spec Ops: The Line and The Darkness 2 are both good games -- a bit short, but the stories are great. If you like strategy games or want to get into one, then Civ 5 is a great place to start, although like others said, you'd probably want to pick up the Gods & Kings expansion to go with it (it adds a lot).
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I have a problem, I don't know which game should I choose! I can get one of them from a trade, and I don't know which one will I like the most. Any Suggestions?
EDIT: I'm trading my copy of GRID on Steam for it. I don't really play RTSes and strategy games, but I heard a lot of good stuff about CIV5. I also heard a lot of good about the rest of those games, too.
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